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• W2026374384 abstract "We probe electronic interaction at molecular-solid/metal interfaces in the model system of C60/Cu(111) using femtosecond two-photon photoemission (2PPE) spectroscopy. The second lowest unoccupied molecular orbital (LUMO+1) and the LUMO+2 levels in C60 are transiently populated via the creation of electronic excitons, with lifetimes in the 10-14−10-13 s region, likely due to self-trapping and/or decay into lower-lying exciton states. These lifetimes decrease as film thickness decreases. The effect is seen for films as thick as 50 Å and is attributed to quenching via charge transfer between the Cu substrate and electronic bands in C60. The rates of quenching are found to depend exponentially on film thickness, with a β value of 0.11 ± 0.02 Å-1 for both LUMO+1 and the LUMO+2 levels." @default.
• W2026374384 created "2016-06-24" @default.
• W2026374384 creator A5005048629 @default.
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• W2026374384 date "2004-05-07" @default.
• W2026374384 modified "2023-10-15" @default.
• W2026374384 title "Distance-Dependent Electronic Coupling at Molecule−Metal Interfaces: C₆₀/Cu(111)" @default.
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• W2026374384 doi "https://doi.org/10.1021/jp036996s" @default.
• W2026374384 hasPublicationYear "2004" @default.
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