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- W2026418419 abstract "The lowest photoexcited triplet state of benzophenone in single crystals of 4,4′-dibromodiphenyl ether has been studied by optically detected ENDOR. The hyperfine coupling tensors for eight protons and carbonyl–13C have been determined by analyzing the angular dependence of the ENDOR spectra. A point–dipole model is presented to account for the anisotropic hyperfine tensor elements based solely on spin densitites and molecular geometry. A set of spin densities and a ring–twist angle have been found which, together, best reproduce the observed dipole interaction tensors as calculated from our model. Data from zero-field ODMR experiments on 17O–benzophenone performed by S. Yamauchi and D. W. Pratt at the University of Pittsburgh enabled us to remove the correlation between n and π spin densities on oxygen. A final fit of all data shows the n electron to be localized on oxygen and the π electron to be delocalized onto the rings." @default.
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- W2026418419 date "1979-03-15" @default.
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- W2026418419 title "Spin densitites in triplet benzophenone" @default.
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