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• W2026470908 abstract "Abstract Photodecomposition of triisobutylaluminum (TIBA) adsorbed on an aluminum surface by pulsed ultraviolet laser irradiation is studied by observing the photoproducts with time-of-flight mass spectroscopy. The fragmentation pattern at different laser wavelengths (193, 248, and 351nm) is very similar and the intensity of fragments at these three wavelengths is 1:0.6:0.05 even though in the gas phase, absorption drops off rapidly for wavelengths above 193nm. In addition, the translational energy of the fragments is considerably less than the photon energy. These findings support a mechanism whereby absorption of light by the surface creates hot electrons which induce desorption of the TIBA molecules, rupture isobutyl groups to create methyl radicals, and induce β-hydride elimination reactions that create isobutylene molecules which desorb from the surface." @default.
• W2026470908 created "2016-06-24" @default.
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• W2026470908 date "1991-01-01" @default.
• W2026470908 modified "2023-09-27" @default.
• W2026470908 title "Evidence for a Charge Transfer Mechanism in Laser Induced Chemical Vapor Deposition" @default.
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• W2026470908 doi "https://doi.org/10.1080/00268949108041161" @default.
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