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- W2026773604 abstract "Direct observation of dynamic equilibrium between preadsorbed $^{13}mathrm{C}$$^{18}mathrm{O}$ and gas phase $^{12}mathrm{C}$$^{16}mathrm{O}$ by means of time-resolved infrared reflection absorption spectroscopy at several temperatures from 350 to 400 K reveals that the desorption process under gas phase CO is enhanced due to the repulsive interaction between preadsorbed $^{13}mathrm{C}$$^{18}mathrm{O}$ and incident $^{12}mathrm{C}$$^{16}mathrm{O}$ molecules from the gas phase arriving at nearby sites of adsorbed CO. As a result, the activation energy is reduced from 127 kJ ${mathrm{mol}}^{ensuremath{-}1}$, the value for desorption into vacuum, to 25 kJ ${mathrm{mol}}^{ensuremath{-}1}$ even for $ensuremath{theta}=0.1ensuremath{-}0.3$ monolayer (ML) and a CO flux of 0.001 ML${mathrm{s}}^{ensuremath{-}1}$." @default.
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- W2026773604 date "1994-07-11" @default.
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- W2026773604 title "Temporal and Local Reduction of a Potential Energy Well under Dynamic Equilibrium: CO on Ni(100)" @default.
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- W2026773604 doi "https://doi.org/10.1103/physrevlett.73.292" @default.
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