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• W2027300704 abstract "Abstract Electronic structure of solid molecular complexes [TPPO 1− x ⋅TPM x ] and [TPPO 1− x ⋅ACN x ] at low temperature (80 K) was investigated by positronium annihilation lifetime spectroscopy (PALS) in order to evaluate the positronium formation at this condition and compare with our previous study recently reported at 294 K. Temporal dependence of the τ 3 ( ortho -positronium lifetime/ns) and I 3 ( ortho -positronium relative intensity/%) at 80 K remained constant throughout the measurement time (10 h), suggesting non-occurrence of electron trapping. The dependence of I 3 with molar fraction at 80 K showed a decrease of I 3 when compared with the values obtained at 294 K (Δ I 3  = 8% for [TPPO 0.5 ⋅TPM 0.5 ] and Δ I 3  = 37% for [TPPO 0.5 ⋅ACN 0.5 ]. These results were rationalized in terms of reduction of electronic availability upon lowering of temperature." @default.
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• W2027300704 date "2015-03-01" @default.
• W2027300704 modified "2023-09-27" @default.
• W2027300704 title "Electronic structure of solid molecular complexes evaluated by positronium formation studies at low temperature" @default.
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• W2027300704 doi "https://doi.org/10.1016/j.molstruc.2014.12.044" @default.
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