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- W2027532634 abstract "Activity coefficients of B in the α phase of Pt and of three PtRh alloys with 3, 6, and 10 wt.% Rh were obtained by equilibration of B2O3 with H2-H2O mixtures between 750 and 1000 °C and subsequent determination of the B mole fraction xB ⩽ 0.06 by the mass gain of the samples or by photometric analysis. Additions of Rh to Pt have rather large but opposing effects on the partial molar enthalpies and entropies of B, resulting in partial molar excess Gibbs energies within the modest range between −40 and −55 kJ mol−1. The change in the lattice contraction from −13.5 to −3.2 pm/xB in the α phase of Pt and of Pt-10Rh can be fully described in terms of a substitutional solution model with strictly constant partial molar volumes of 9.09 cm3 mol−1 and 8.28 cm3 mol−1 for Pt and Rh respectively and a partial molar volume for B that increases linearly from 8.2 to 8.9 cm3 mol−1 between pure Pt and Pt-10Rh." @default.
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- W2027532634 date "1995-04-01" @default.
- W2027532634 modified "2023-09-27" @default.
- W2027532634 title "Activity coefficients and partial molar volumes of boron in platinum-rhodium alloys" @default.
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- W2027532634 doi "https://doi.org/10.1016/0925-8388(94)06011-8" @default.
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