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- W2027831964 abstract "Abstract A critical review of the data available on the oxidation of uranium in carbon dioxide and carbon monoxide is presented. The basic uranium-carbon dioxide reaction results in the production of uranium dioxide which, depending on the oxidation temperature, contains small quantities of free or combined carbon. Up to ~700 °C the reaction is controlled by O 2− ion diffusion through a layer of oxide next to the metal. Above this temperature, however, the mechanism is uncertain due to the formation of a multilayer product and to difficulties in obtaining reliable isothermal data. Variations in the purity of the carbon dioxide or the metallurgical condition of the uranium affect the oxidation rate in the α-phase but become insignificant at higher temperatures. Data on the reaction of uranium with carbon monoxide are more limited. The principal products are uranium dioxide and uranium dicarbide and it is evident that the mechanism is complex and not well established. Similarly, the effects of irradiation during oxidation in carbon dioxide or carbon monoxide have not been fully investigated although the data available suggest that the oxidation rates are not appreciably enhanced." @default.
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- W2027831964 date "1969-10-01" @default.
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- W2027831964 title "The oxidation of uranium in carbon dioxide and carbon monoxide (A review)" @default.
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- W2027831964 doi "https://doi.org/10.1016/0022-3115(69)90002-6" @default.
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