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- W2027888946 abstract "The ultraviolet photodissociation of 1-bromo-3-fluorobenzene and 1-bromo-4-fluorobenzene at 266 nm has been performed on a universal crossed molecular beams machine combined with the photofragment translational spectroscopy (PTS) detection technique. The time-of-flight (TOF) spectra of Br and FC6H4 photofragments have been measured. The observed translational energy distributions P(Et) of photofragments revealed that about 46.8 ± 3.3% and 41.7 ± 3.0% of the available energy are partitioned into translational energy and the anisotropy parameter β is 0.7 ± 0.1 and −0.4 ± 0.1 for 1-bromo-3-fluorobenzene and 1-bromo-4-fluorobenzene, in accord with that of bromobenzene (−0.7), indicating significant change caused by the fluorine atom substitution. To better interpret the experimental results, ab initio calculations have been performed and the calculation results are in good agreement with the experimental results. A plausible photodissociation mechanism is suggested, and the substitution effect of the fluorine atom is discussed." @default.
- W2027888946 created "2016-06-24" @default.
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- W2027888946 date "2000-12-22" @default.
- W2027888946 modified "2023-10-12" @default.
- W2027888946 title "Photofragment Translational Spectroscopy of 1-Bromo-3-fluorobenzene and 1-Bromo-4-fluorobenzene at 266 nm" @default.
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- W2027888946 doi "https://doi.org/10.1021/jp003479q" @default.
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