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• W2027890346 abstract "In-situ spectroscopic ellipsometry is used for the dynamic study of thermally perturbed thin polystyrene films, swollen with n-octane or n-decane. The thermal evolution of the swollen films reveals pronounced changes both in equilibrium and kinetic properties. Upon vitrification, a kinetically arrested swollen matrix is observed. This phenomenon is related to the excess energy term in the chemical potential of the solvent, associated with the non-equilibrium status of the swollen polymer matrix. The swollen polystyrene – n-decane system shows no measurable compression when exposed to hydrostatic pressures up to 50 bar, neither above or below the glass transition temperature. A slight compression is observed for a glassy polystyrene film in pressurized water. This compression corresponds to partial relaxation of excess free volume. The results are of importance for membrane applications in which penetrant-swollen polymer membrane layers are operated under high pressures." @default.
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• W2027890346 date "2014-08-01" @default.
• W2027890346 modified "2023-09-27" @default.
• W2027890346 title "Effects of time, temperature, and pressure in the vicinity of the glass transition of a swollen polymer" @default.
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• W2027890346 doi "https://doi.org/10.1016/j.memsci.2014.04.013" @default.
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