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- W2028065889 abstract "A uniform theory of photo-emission from a dissociating molecule excited by a laser pulse is used to decipher the recently observed CH3I emission signal as a function of the excitation wavelength (“excitation-emission” spectrum). The theory, which incorporates transient effects not included in the Kramers—Heisenberg formula, uniformly interpolates between the “true” Raman and “resonance fluorescence” limits. Computations of the transient and time-averaged excitation-emission spectrum of CH3I with pulses of different durations (spanning the fs to ns range) are presented. The present study explains the rich structure observed experimentally with ns pulses and points out ways of translating this structure to “real-time” information." @default.
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- W2028065889 date "1993-09-01" @default.
- W2028065889 modified "2023-09-23" @default.
- W2028065889 title "Theory of the continuum excitation-emission spectrum of CH3I" @default.
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- W2028065889 doi "https://doi.org/10.1016/0009-2614(93)87226-s" @default.
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