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• W2028101067 abstract "The triple “magnetic−transport−structural” transition versus temperature in three series of “114” cobaltites, Y1−xYbxBaCo4O7, Y1−xCaxBaCo4O7, and Yb1−xCaxBaCo4O7, has been studied using magnetic, transport, and differential scanning calorimetric measurements. The effect of the size mismatch σ2, because of cationic disordering at the Ln sites upon such a transition is shown for the first time in a triangular lattice. We show that increasing ⟨rLn⟩ has an effect of increasing TS dramatically, while the size mismatch σ2 at the Ln sites decreases TS substantially. Moreover, the cationic mismatch at the Ln sites modifies the nature of the hysteretic transition by turning the sharp first-order transition seen in the undoped samples into an intermix of first and second-order transitions. These results are discussed on the basis of the particular nature of the high-temperature form that exhibits a hexagonal close packed structure (space group P63mc) with respect to the low-temperature orthorhombic form (space group Pbn21), the latter corresponding to a distortion of the former because of a puckering of the kagomé layers." @default.
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• W2028101067 date "2010-11-12" @default.
• W2028101067 modified "2023-09-25" @default.
• W2028101067 title "Hysteretic “Magnetic−Transport−Structural” Transition in “114” Cobaltites: Size Mismatch Effect" @default.
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• W2028101067 doi "https://doi.org/10.1021/cm103088e" @default.
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