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- W2028120164 endingPage "6390" @default.
- W2028120164 startingPage "6369" @default.
- W2028120164 abstract "The vibrational structures observed in the absorption spectrum associated with the crystal-field transitions in Mn, Fe, Co, and Ni dichlorides and dibromides are studied in detail at 5 K. The choice of these crystals is motivated by their appreciable molecular character resulting in a small dispersion of optical branches and hence in the appearance of relatively sharp phonon progressions in the crystal-field spectra. Most of these phonon structures are replicas of Raman-active ${A}_{1g}$ and ${E}_{g}$ frequencies and readily interpreted in terms of many-phonon processes induced by the first-order linear electron-phonon interaction. Furthermore, in Mn and Ni dihalides some intraconfigurational transitions display interesting two-phonon progressions which are attributed to the second-order linear electron-phonon interaction. The $q=0$ phonon frequencies of even symmetry, deduced from vibronic or Raman spectra, and those of odd symmetry, measured by far-infrared transmission, are interpreted in the framework of a deformation-dipole model. Information on the partial covalency of these compounds and on the magnitude of three-body interactions is derived." @default.
- W2028120164 created "2016-06-24" @default.
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- W2028120164 date "1980-12-15" @default.
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- W2028120164 title "Vibrational structure of crystal-field spectra in layered<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mn>3</mml:mn><mml:mi>d</mml:mi></mml:math>-metal dihalides" @default.
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- W2028120164 doi "https://doi.org/10.1103/physrevb.22.6369" @default.
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