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- W2028254674 abstract "Using a new approach, Stauffer’s expression for the rate of steady state binary nucleation and Trinkaus’s expression for the steady state cluster concentrations f are derived directly from the diffusion equation that governs the evolution of f in composition space. The behavior of Φ (≡f/N, where N is the equilibrium cluster concentration) is explored since this function provides a characterization of the nucleating binary system that, to lowest order, is independent of the actual composition of the mother phase. The angle ω that describes the direction of ∇Φ at the saddle point differs, in general, from the angle φ found by Stauffer for the direction of the nucleation current at the saddle point. These two angles are related by the formula: tan φ=r tan ω, where r is the ratio of impingement frequencies defined by Stauffer. In general, at the saddle point, ∇Φ also fails to lie in the direction of steepest descent on the free energy surface." @default.
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- W2028254674 date "1999-04-01" @default.
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- W2028254674 title "Binary nucleation kinetics. IV. Directional properties and cluster concentrations at the saddle point" @default.
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- W2028254674 doi "https://doi.org/10.1063/1.478547" @default.
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