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• W2028305118 abstract "Abstract Resonance Raman spectra excited at 458 and 476 nm are reported for [Ru(bipyridine) 3 ] 2+ in water, acetonitrile and their perdeuterated derivatives. Raman intensities of [Ru(bipyridine) 3 ] 2+ are about a factor of two greater in H 2 O than D 2 O for all vibrational modes, but are independent of solvent isotopomer in acetonitrile. Solvent dynamics apparently contribute more strongly to the dephasing dynamics in water than in acetonitrile. Mode‐specific dephasing rates seem to cause different depolarization ratios for different observed vibrations which can lead to a potentially misleading interpretation of the depolarization ratios. We speculate that a static complex between [Ru(bipyridine) 3 ] 2+ and water influences the excited‐state dynamics. Copyright © 2001 John Wiley & Sons, Ltd." @default.
• W2028305118 created "2016-06-24" @default.
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• W2028305118 date "2001-06-01" @default.
• W2028305118 modified "2023-10-03" @default.
• W2028305118 title "Resonance Raman spectrum of [Ru(bipyridine)₃]²⁺ in water, acetonitrile and their deuterated derivatives: the possible role of solvent in excited‐state charge localization" @default.
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• W2028305118 doi "https://doi.org/10.1002/jrs.733" @default.
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