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- W2028326228 abstract "Catalytic multicomponent [m + n + o]-type cycloadditions offer efficient, atom-economical routes to diverse complex carbocycles. Recently, such transformations have emerged as unique strategies for medium ring carbocycle synthesis. Despite the important developments in this area, however, highly enantioselective [m + n + o]-type processes accessing medium ring carbocycles have yet to be developed. Herein, a rhodium-catalyzed [4 + 2 + 2] cycloaddition of allenedienes with allenes enabling the direct stereoselective synthesis of cis-fused cyclooctanoids is reported. These cycloadditions are successful with a diverse range of π-components and demonstrate the potential for high levels of enantioselectivity in a [4 + 2 + 2] process." @default.
- W2028326228 created "2016-06-24" @default.
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- W2028326228 date "2015-02-18" @default.
- W2028326228 modified "2023-09-27" @default.
- W2028326228 title "Enantioselective Synthesis of cis-Fused Cyclooctanoids via Rhodium(I)-Catalyzed [4 + 2 + 2] Cycloadditions" @default.
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- W2028326228 doi "https://doi.org/10.1021/acs.orglett.5b00267" @default.
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