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- W2028495521 abstract "Previous optical second harmonic generation (SHG) studies of single domain Si(111)-4x1-In revealed a large in-surface-plane optical anisotropy, with an enhanced hyperpolarisability aligned along the In chains. This single wavelength study indicated that SHG might provide a non-contact, non-destructive method of characterising low dimensional metallic behaviour. However, it was not clear whether the observed enhancement is due to the low dimensional metallicity, or to the presence of surface and interface states at either the fundamental or SH energy. Spectroscopic SHG studies from single domain Si(111)-4x1-In are reported. A very large anisotropy in the SH response is observed using excitation energies in the 1.36-1.65 eV region, with the dominant hyperpolarizability orthogonal to the chain direction. The results help to clarify the approach likely to be necessary to use SHG as a probe of low dimensional metallic behaviour on planar surfaces. (© 2003 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim)" @default.
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- W2028495521 date "2003-12-01" @default.
- W2028495521 modified "2023-10-16" @default.
- W2028495521 title "Anisotropic second harmonic generation from Si(111)-4x1-In" @default.
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- W2028495521 doi "https://doi.org/10.1002/pssc.200303832" @default.
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