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- W2028593460 abstract "A new structure for the cytotoxic cembranolide uprolide F diacetate (UFD) was proposed, and an enantioselective total synthesis was accomplished to confirm that our revised structure correctly represented the natural UFD and its absolute configuration. Our synthesis features a late-stage, highly efficient, and diastereoselective Nozaki-Hiyama-Kishi macrocyclization (95% yield) and an unexpected reagent-controlled reversible translactonization, which, being the first example within the cembranolide family, might have biogenetic implications and be of great importance to synthetic studies of the α-methylene-γ-lactone-bearing cembranolides." @default.
- W2028593460 created "2016-06-24" @default.
- W2028593460 creator A5020424168 @default.
- W2028593460 creator A5042455393 @default.
- W2028593460 date "2015-04-01" @default.
- W2028593460 modified "2023-10-18" @default.
- W2028593460 title "Structural Revision of (+)-Uprolide F Diacetate Confirmed by Asymmetric Total Synthesis" @default.
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- W2028593460 doi "https://doi.org/10.1021/acs.orglett.5b00700" @default.
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