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- W2028857710 abstract "Abstract Hydrogen sulfide (H 2 S) methane (CH 4 ) reformation (H 2 SMR) (2H 2 S + CH 4 = CS 2 + 4H 2 ) is a potentially viable process for the removal of H 2 S from sour natural gas resources or other methane containing gases. Unlike steam methane reformation that generates carbon dioxide as a by-product, H 2 SMR produces carbon disulfide (CS 2 ), a liquid under ambient temperature and pressure—a commodity chemical that is also a feedstock for the synthesis of sulfuric acid. Pinch point analyses for H 2 SMR were conducted to determine the reaction conditions necessary for no carbon lay down to occur. Calculations showed that to prevent solid carbon formation, low inlet CH 4 to H 2 S ratios are needed. In this paper, we analyze H 2 SMR with either a cryogenic process or a membrane separation operation for production of either liquid or gaseous hydrogen. Of the three H 2 SMR hydrogen production flowsheets analyzed, direct liquid hydrogen generation has higher first and second law efficiencies of exceeding 80% and 50%, respectively." @default.
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- W2028857710 date "2008-01-01" @default.
- W2028857710 modified "2023-09-27" @default.
- W2028857710 title "Liquid hydrogen production via hydrogen sulfide methane reformation" @default.
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- W2028857710 doi "https://doi.org/10.1016/j.jpowsour.2007.09.079" @default.
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