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• W2028874736 abstract "Pd was loaded on ultra stable Y (USY) zeolites prepared by steaming NH4-Y zeolite under different conditions. Heck reactions were carried out over the prepared Pd/USY. We found that H2 bubbling was effective in improving not only the catalytic activity of Pd/USY, but also that of other supported Pd catalysts and Pd(OAc)2. Moreover, the catalytic activity of Pd/USY could be optimized by choosing appropriate steaming conditions for the preparation of the USY zeolites; Pd loaded on USY prepared at 873 K with 100% H2O gave the highest activity (TOF = 61,000 h−1), which was higher than that of Pd loaded on other kinds of supports. The prepared Pd/USY catalysts were applicable to the Heck reactions using various kinds of substrates including bromo- and chloro-substituted aromatic and heteroaromatic compounds. Characterization of the acid properties of the USY zeolites revealed that the strong acid site (OHstrong) generated as a result of steaming had a profound effect on the catalytic activity of Pd." @default.
• W2028874736 created "2016-06-24" @default.
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• W2028874736 date "2010-12-24" @default.
• W2028874736 modified "2023-09-29" @default.
• W2028874736 title "Enhancement in the Catalytic Activity of Pd/USY in the Heck Reaction Induced by H2 Bubbling" @default.
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• W2028874736 doi "https://doi.org/10.3390/molecules16010038" @default.
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