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• W2029123342 endingPage "406" @default.
• W2029123342 startingPage "401" @default.
• W2029123342 abstract "Measurements of the nascent OH product from photodissociation of gaseous nitromethane and nitroethane at 266 nm were performed using the single-photon laser induced fluorescence technique. The OH fragment is found to be vibrationally cold for both systems. The rotational state distribution of nitromethane are Boltzmann, with rotational temperature of Trot=2045150 and 1923150 K for both 23/2 and 21/2 states, respectively. For nitroethane, the rotational state distribution shows none Boltzmann and cannot be well characterized by a rotational temperature, which indicates the different mechanisms in producing OH radicals from photodissociation of nitromethane and nitroethane. The rotational energy is calculated as 14.360.8 and 4.980.8 kJ/mol for nitromethane and nitroethane, respectively. A preferential population of the low spin-orbit component (23/2) is observed for both nitromethane and nitroethane. The dominant population of + state in two -doublet states is also observed for both nitromethane and nitroethane, which indicates that the unpaired lobe of the OH fragment is parallel to the plane of rotation." @default.
• W2029123342 created "2016-06-24" @default.
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• W2029123342 date "2007-08-01" @default.
• W2029123342 modified "2023-10-16" @default.
• W2029123342 title "Photodissociation Dynamics of Nitromethane and Nitroethane at 266 nm" @default.
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• W2029123342 doi "https://doi.org/10.1088/1674-0068/20/04/401-406" @default.
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