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- W2029138860 abstract "The two-photon vapor Ã←X̃ spectra of benzonitrile and styrene have been studied by fluorescence excitation at room temperature. Because of low frequency internal torsional vibrations, the styrene spectrum was also obtained using multiphoton ionization in a supersonic jet. Despite the totally symmetric symmetry of the excited state, the polarization properties of the styrene Franck–Condon spectrum show that the two-photon electronic intensity mechanism predominantly involves the symmetric tensor and not the scalar tensor. Comparison with the corresponding 1B2←1A1 spectrum of phenylacetylene shows that the cross section for the two-photon spectra of the three molecules are roughly equal (∼102 gm) despite a large dissimilarity in the one-photon spectra. The near equality of the three cross sections in molecules without special symmetry properties confirms both the pseudoparity (±) basis of the Callis–Scott–Albrecht inductive perturbation selection rule, and the rule that orbitally allowed -↔- transitions should be very strong for alternant aromatic hydrocarbon two-photon spectra." @default.
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- W2029138860 date "1983-07-15" @default.
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- W2029138860 title "Two‐photon <i>A</i>̃←<i>X</i>̃ spectra of benzonitrile and styrene vapors: Tests of perturbation rules" @default.
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- W2029138860 doi "https://doi.org/10.1063/1.445806" @default.
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