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• W2029144464 abstract "The formation of Ar and H2 clusters, having up to 900 particles in helium droplets, has been studied via laser induced fluorescence of attached Mg-phthalocyanine (Mg-Pc) molecules. In the experiments, one Mg-Pc molecule in average was added to each He droplet either before or after the cluster species, and the shift of the spectrum of the Mg-Pc molecules was studied as a function of the cluster size. For Ar clusters, about a factor of 2 smaller matrix shift was observed for the late pickup of the Mg-Pc molecules as compared with the prior pickup, indicating that in the former case, the Mg-Pc molecules reside on the surface of the preformed Ar clusters. On the other hand, the spectra of the Mg-Pc molecules attached to H2 clusters are independent of the pickup order, which is consistent with Mg-Pc molecules residing near the center of the H2 clusters in both cases. Therefore H2 clusters remain fluxional in helium droplets at T=0.38 K. No significant differences in the spectra were observed between the para-H2 and ortho-H2 clusters." @default.
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• W2029144464 date "2007-12-03" @default.
• W2029144464 modified "2023-09-28" @default.
• W2029144464 title "Laser induced fluorescence of Mg-phthalocyanine in He droplets: Evidence for fluxionality of large H2 clusters at 0.38K" @default.
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• W2029144464 doi "https://doi.org/10.1063/1.2802303" @default.
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