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• W2029190497 abstract "Near-edge X-ray absorption fine structure (NEXAFS) spectroscopy and microscopy has been used to study the orientational morphology of thin films of the linear alkanes n-C36H74 and n-C60H122, prepared by vacuum deposition onto NaCl (001) surfaces at ambient and elevated substrate temperatures. The orientational morphology, specifically, the nature of domains with lateral and normal orientation, is explored as a function of the chain length and the substrate temperature. It is found that the longer n-C60H122 molecules are laterally oriented on the substrate surface within the investigated substrate temperatures but that the morphology of these thin films varies with substrate temperature. The shorter n-C36H74 molecules are partially laterally oriented at low substrate temperature and are completely normally oriented at high substrate temperature. The relative magnitude of “side-by-side” and “end-to-end” intermolecular interactions leads to the formation of highly ordered alkane structures with a high aspect ratio. The formation of complex, nanoscale orientational morphologies are rationalized by considering kinetic and thermodynamic effects, in particular, the relative enthalpic and entropic contributions to the free energy associated with the different molecular orientations." @default.
• W2029190497 created "2016-06-24" @default.
• W2029190497 creator A5019137551 @default.
• W2029190497 creator A5076908097 @default.
• W2029190497 date "2007-02-01" @default.
• W2029190497 modified "2023-10-12" @default.
• W2029190497 title "Effect of Chain Length and Substrate Temperature on the Growth and Morphology of <i>n</i>-Alkane Thin Films" @default.
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• W2029190497 doi "https://doi.org/10.1021/la0630007" @default.
• W2029190497 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/17266340" @default.
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