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• W2029273119 endingPage "6927" @default.
• W2029273119 startingPage "6924" @default.
• W2029273119 abstract "Radicals in directed pathways: The μ-η2:η2 peroxo CuII2 intermediate 1 shows a much faster benzylic ligand hydroxylation than systems without phenol. This novel reactivity can be further accelerated by addition of external H-atom donors such as TEMPO-H. The results imply initial H-atom transfer leading to the formation of phenoxyl radicals. A highly reactive copper oxyl intermediate is then formed, which inserts oxygen into the benzylic CH bond." @default.
• W2029273119 created "2016-06-24" @default.
• W2029273119 creator A5063000822 @default.
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• W2029273119 date "2011-06-17" @default.
• W2029273119 modified "2023-10-18" @default.
• W2029273119 title "Benzylic Ligand Hydroxylation Starting from a Dicopper μ-η2:η2 Peroxo Intermediate: Dramatic Acceleration of the Reaction by Hydrogen-Atom Donors" @default.
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• W2029273119 doi "https://doi.org/10.1002/anie.201102332" @default.
• W2029273119 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/21688374" @default.
• W2029273119 hasPublicationYear "2011" @default.
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