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• W2029450521 startingPage "1903" @default.
• W2029450521 abstract "A kinetic theory description of a dense chemically reacting fluid is presented. The kinetic equation takes into account the effects of correlated binary collision events and involves the ’’repeated ring’’ operator. Expressions for the rate coefficient are derived from the kinetic equation by means of projection operator techniques. The resulting expressions for the rate coefficient incorporate several features. They show how the dynamics of the reactive collision events lead to a coupling to the diffusive modes of the fluid. The rate coefficient expression is valid in the limit where binary dynamics dominate as well as in the diffusion controlled limit where collective solvent effects play an important role. The frequency and time dependence of the rate kernels and rate coeffiicients are also calculated. The manner in which the kinetic theory can be used to take into account the contributions to the rate coefficient which are higher order in the concentration is described and the relation to other theories is discussed." @default.
• W2029450521 created "2016-06-24" @default.
• W2029450521 creator A5041147881 @default.
• W2029450521 date "1978-02-15" @default.
• W2029450521 modified "2023-10-16" @default.
• W2029450521 title "Kinetic theory of chemical reactions in dense fluids" @default.
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• W2029450521 doi "https://doi.org/10.1063/1.435917" @default.
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