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- W2029467625 abstract "Laser flash photolysis of SiCl4 at 193 nm was studied behind reflected shock waves at temperatures 1000 K ≤ T ≤ 2050 K and pressures between 1.4 and 1.8 bar. The atomic resonance absorption spectroscopy (ARAS) was applied for time-resolved measurements of Si- and Cl-atom concentrations in gas mixtures containing 10−100 ppm SiCl4 highly diluted in argon. The atoms formed during photolysis of SiCl4 were analyzed in terms of yields, defined as the fractions of the maximum atom concentration to the initial SiCl4 concentration behind the shock wave. At temperatures 1000 ≤ T ≤ 1510 K, Cl atoms were detected immediately after the laser flash. The Cl yield was found to be temperature dependent in the range between 0.1 and 2% of the initial SiCl4 concentration. Si atoms first occurred at temperatures T > 1750 K, when SiCl4 already has started to decompose. In contrast to Cl, the Si yield obtained correlates with both the temperature and the delay time between the shock-induced gas heating and the laser pulse. This..." @default.
- W2029467625 created "2016-06-24" @default.
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- W2029467625 date "2010-06-16" @default.
- W2029467625 modified "2023-09-25" @default.
- W2029467625 title "ChemInform Abstract: Laser Flash Photolysis of SiCl4 at High Temperatures Based on Si- and Cl-Concentration Measurements." @default.
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- W2029467625 doi "https://doi.org/10.1002/chin.199918018" @default.
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