Matches in SemOpenAlex for { <https://semopenalex.org/work/W2029522056> ?p ?o ?g. }
- W2029522056 abstract "We propose a process to convert ultracold metastable ${mathrm{Cs}}_{2}$ molecules in their lowest triplet state into (singlet) ground-state molecules in their lowest vibrational levels. Molecules are first pumped into an excited triplet state, and the triplet-singlet conversion is facilitated by a two-step spontaneous decay through the coupled $A {}^{1}{ensuremath{Sigma}}_{u}^{+}ensuremath{-}b {}^{3}{ensuremath{Pi}}_{u}$ states. Using spectroscopic data and accurate quantum chemistry calculations for ${mathrm{Cs}}_{2}$ potential curves and transition dipole moments, we show that this process competes favorably with the single-photon decay back to the lowest triplet state. In addition, we demonstrate that this conversion process represents a loss channel for vibrational cooling of metastable triplet molecules, preventing an efficient optical pumping cycle down to low vibrational levels." @default.
- W2029522056 created "2016-06-24" @default.
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- W2029522056 date "2011-02-08" @default.
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- W2029522056 title "Triplet-singlet conversion in ultracold<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mi mathvariant=normal>Cs</mml:mi><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>and production of ground-state molecules" @default.
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- W2029522056 doi "https://doi.org/10.1103/physreva.83.022503" @default.
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