Matches in SemOpenAlex for { <https://semopenalex.org/work/W2029550043> ?p ?o ?g. }
- W2029550043 endingPage "5324" @default.
- W2029550043 startingPage "5313" @default.
- W2029550043 abstract "An important issue for developing a molecular-level mechanism of heterogeneous interactions at the aqueous interface is determining changes in the interface with changes in the bulk composition. Development of the nonlinear spectroscopy, sum frequency generation (SFG) provides a technique to probe these changes. Several molecular and ionic solutes have been used to investigate changes in the structure of the aqueous interface. Molecular solutes include glycerol and ammonia. Ionic and associated ion complexes include sulfuric acid as well as alkali sulfate and bisulfate salts. Molecular solutes and associated ion complexes penetrate to the top monolayer of the aqueous-air interface displacing water from the interface. Specifically, the conjectured ammonia−water complex is observed with ammonia tilted, on average, 25−38° from the normal. Ionic solutes generate a double layer in the interfacial region due to the differential distribution of anions and cations near the interface. The strength of the double layer is dependent on ion size and charge. Due to the extreme size of the proton, the strongest field is generated by acidic solutes. As the ionic solute concentration increases, associated ion pairs form and these penetrate to the top monolayer. These results have wide implications because the aqueous interface is ubiquitous in atmospheric and biological systems." @default.
- W2029550043 created "2016-06-24" @default.
- W2029550043 creator A5020412802 @default.
- W2029550043 creator A5025045207 @default.
- W2029550043 creator A5058640735 @default.
- W2029550043 creator A5091584020 @default.
- W2029550043 date "2002-05-04" @default.
- W2029550043 modified "2023-10-10" @default.
- W2029550043 title "Aqueous Solution/Air Interfaces Probed with Sum Frequency Generation Spectroscopy" @default.
- W2029550043 cites W1593655292 @default.
- W2029550043 cites W1966571511 @default.
- W2029550043 cites W1968003297 @default.
- W2029550043 cites W1968638792 @default.
- W2029550043 cites W1970928683 @default.
- W2029550043 cites W1971084657 @default.
- W2029550043 cites W1974987639 @default.
- W2029550043 cites W1975329699 @default.
- W2029550043 cites W1975805501 @default.
- W2029550043 cites W1976256678 @default.
- W2029550043 cites W1978544368 @default.
- W2029550043 cites W1979657804 @default.
- W2029550043 cites W1982206363 @default.
- W2029550043 cites W1982385940 @default.
- W2029550043 cites W1982677968 @default.
- W2029550043 cites W1983152402 @default.
- W2029550043 cites W1987152262 @default.
- W2029550043 cites W1987692212 @default.
- W2029550043 cites W1988069708 @default.
- W2029550043 cites W1988396543 @default.
- W2029550043 cites W1989084891 @default.
- W2029550043 cites W1991098454 @default.
- W2029550043 cites W1991452898 @default.
- W2029550043 cites W1994014080 @default.
- W2029550043 cites W1998056750 @default.
- W2029550043 cites W1998116533 @default.
- W2029550043 cites W1998608330 @default.
- W2029550043 cites W2000827899 @default.
- W2029550043 cites W2001651483 @default.
- W2029550043 cites W2003066948 @default.
- W2029550043 cites W2004472642 @default.
- W2029550043 cites W2004799172 @default.
- W2029550043 cites W2006583700 @default.
- W2029550043 cites W2007018151 @default.
- W2029550043 cites W2011985909 @default.
- W2029550043 cites W2012520426 @default.
- W2029550043 cites W2013387328 @default.
- W2029550043 cites W2017674438 @default.
- W2029550043 cites W2018697447 @default.
- W2029550043 cites W2019645025 @default.
- W2029550043 cites W2021246523 @default.
- W2029550043 cites W2026174057 @default.
- W2029550043 cites W2031814529 @default.
- W2029550043 cites W2032463519 @default.
- W2029550043 cites W2033273396 @default.
- W2029550043 cites W2035971133 @default.
- W2029550043 cites W2041135698 @default.
- W2029550043 cites W2041703304 @default.
- W2029550043 cites W2043373656 @default.
- W2029550043 cites W2044600799 @default.
- W2029550043 cites W2045211165 @default.
- W2029550043 cites W2046847095 @default.
- W2029550043 cites W2047220791 @default.
- W2029550043 cites W2050501604 @default.
- W2029550043 cites W2051630390 @default.
- W2029550043 cites W2053315875 @default.
- W2029550043 cites W2053659908 @default.
- W2029550043 cites W2054414697 @default.
- W2029550043 cites W2060814251 @default.
- W2029550043 cites W2063342489 @default.
- W2029550043 cites W2064932773 @default.
- W2029550043 cites W2068096872 @default.
- W2029550043 cites W2068304618 @default.
- W2029550043 cites W2068935762 @default.
- W2029550043 cites W2069366616 @default.
- W2029550043 cites W2070451289 @default.
- W2029550043 cites W2071467656 @default.
- W2029550043 cites W2072592896 @default.
- W2029550043 cites W2072810218 @default.
- W2029550043 cites W2075614487 @default.
- W2029550043 cites W2076598330 @default.
- W2029550043 cites W2079493449 @default.
- W2029550043 cites W2081265484 @default.
- W2029550043 cites W2081926166 @default.
- W2029550043 cites W2082003750 @default.
- W2029550043 cites W2083407560 @default.
- W2029550043 cites W2088960562 @default.
- W2029550043 cites W2098149420 @default.
- W2029550043 cites W2108363120 @default.
- W2029550043 cites W2109537480 @default.
- W2029550043 cites W2121242766 @default.
- W2029550043 cites W2155883293 @default.
- W2029550043 cites W2158110334 @default.
- W2029550043 cites W2161675628 @default.
- W2029550043 cites W2164701295 @default.
- W2029550043 cites W2165372810 @default.
- W2029550043 cites W2249980874 @default.
- W2029550043 cites W2315470425 @default.
- W2029550043 cites W2316319537 @default.