FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W2029567090> ?p ?o ?g. }

• W2029567090 endingPage "2455" @default.
• W2029567090 startingPage "2441" @default.
• W2029567090 abstract "The dynamics of uv/visible laser-induced nonthermal desorption of neutral molecules from metal surfaces are studied by Liouville–von Neumann equations for quantum open systems. A one-dimensional, two-state Gadzuk–Antoniewicz model is adopted, representative for NO/Pt(111). Electronic quenching due to coupling of the adsorbate negative ion resonance to the metal electrons is treated within the Lindblad dynamical semigroup approach. Both indirect (hot-electron mediated) and hypothetical direct (dipole) excitation processes are considered. For the indirect pathways, DIET (single-excitation) and DIMET (multiple-excitation) limits are studied using one- and double-dissipative channel models, respectively. To reproduce experimental desorption yields and desorbate translational energies, we estimate the quenching lifetime for NO/Pt(111) to be less than 5 fs. We also extend previous quantum treatments of photodesorption processes to the case of coordinate-dependent quenching rates. Further, the characteristic scaling laws of desorption yields versus laser fluence are derived for each of the individual excitation pathways. Finally, the possibility to control photoreactivity at surfaces by different, vibration-promoted schemes (surface heating, ir+uv two-photon strategies, use of pulsed uv lasers) is examined." @default.
• W2029567090 created "2016-06-24" @default.
• W2029567090 creator A5061906414 @default.
• W2029567090 creator A5086549023 @default.
• W2029567090 date "1996-08-08" @default.
• W2029567090 modified "2023-10-17" @default.
• W2029567090 title "Quantum dynamics of bond breaking in a dissipative environment: Indirect and direct photodesorption of neutrals from metals" @default.
• W2029567090 cites W1964134368 @default.
• W2029567090 cites W1965707657 @default.
• W2029567090 cites W1966162943 @default.
• W2029567090 cites W1969619344 @default.
• W2029567090 cites W1970909917 @default.
• W2029567090 cites W1972975831 @default.
• W2029567090 cites W1976444423 @default.
• W2029567090 cites W1984623004 @default.
• W2029567090 cites W1990766352 @default.
• W2029567090 cites W1991467329 @default.
• W2029567090 cites W1992449867 @default.
• W2029567090 cites W1992813446 @default.
• W2029567090 cites W1993140575 @default.
• W2029567090 cites W1994314374 @default.
• W2029567090 cites W1995459299 @default.
• W2029567090 cites W1996303459 @default.
• W2029567090 cites W1996751821 @default.
• W2029567090 cites W2003177179 @default.
• W2029567090 cites W2003473531 @default.
• W2029567090 cites W2012192021 @default.
• W2029567090 cites W2012482563 @default.
• W2029567090 cites W2015683881 @default.
• W2029567090 cites W2024918335 @default.
• W2029567090 cites W2025168551 @default.
• W2029567090 cites W2026008088 @default.
• W2029567090 cites W2028847674 @default.
• W2029567090 cites W2031473369 @default.
• W2029567090 cites W2032839191 @default.
• W2029567090 cites W2042271158 @default.
• W2029567090 cites W2042720969 @default.
• W2029567090 cites W2044401631 @default.
• W2029567090 cites W2046546342 @default.
• W2029567090 cites W2053290544 @default.
• W2029567090 cites W2054957755 @default.
• W2029567090 cites W2055851286 @default.
• W2029567090 cites W2058324353 @default.
• W2029567090 cites W2064478299 @default.
• W2029567090 cites W2066492928 @default.
• W2029567090 cites W2073019097 @default.
• W2029567090 cites W2073756993 @default.
• W2029567090 cites W2074193845 @default.
• W2029567090 cites W2085295404 @default.
• W2029567090 cites W2086081708 @default.
• W2029567090 cites W2087478059 @default.
• W2029567090 cites W2088925773 @default.
• W2029567090 cites W2089736410 @default.
• W2029567090 cites W2090491132 @default.
• W2029567090 cites W2090985134 @default.
• W2029567090 cites W2091764752 @default.
• W2029567090 cites W2107982977 @default.
• W2029567090 cites W2157495649 @default.
• W2029567090 doi "https://doi.org/10.1063/1.472112" @default.
• W2029567090 hasPublicationYear "1996" @default.
• W2029567090 type Work @default.
• W2029567090 sameAs 2029567090 @default.
• W2029567090 citedByCount "118" @default.
• W2029567090 countsByYear W20295670902012 @default.
• W2029567090 countsByYear W20295670902013 @default.
• W2029567090 countsByYear W20295670902018 @default.
• W2029567090 countsByYear W20295670902019 @default.
• W2029567090 countsByYear W20295670902020 @default.
• W2029567090 countsByYear W20295670902021 @default.
• W2029567090 countsByYear W20295670902023 @default.
• W2029567090 crossrefType "journal-article" @default.
• W2029567090 hasAuthorship W2029567090A5061906414 @default.
• W2029567090 hasAuthorship W2029567090A5086549023 @default.
• W2029567090 hasConcept C121332964 @default.
• W2029567090 hasConcept C121745418 @default.
• W2029567090 hasConcept C147120987 @default.
• W2029567090 hasConcept C147789679 @default.
• W2029567090 hasConcept C150394285 @default.
• W2029567090 hasConcept C159467904 @default.
• W2029567090 hasConcept C162711632 @default.
• W2029567090 hasConcept C184779094 @default.
• W2029567090 hasConcept C185592680 @default.
• W2029567090 hasConcept C41999313 @default.
• W2029567090 hasConcept C62520636 @default.
• W2029567090 hasConcept C83581075 @default.
• W2029567090 hasConcept C91881484 @default.
• W2029567090 hasConcept C99692599 @default.
• W2029567090 hasConceptScore W2029567090C121332964 @default.
• W2029567090 hasConceptScore W2029567090C121745418 @default.
• W2029567090 hasConceptScore W2029567090C147120987 @default.
• W2029567090 hasConceptScore W2029567090C147789679 @default.
• W2029567090 hasConceptScore W2029567090C150394285 @default.
• W2029567090 hasConceptScore W2029567090C159467904 @default.
• W2029567090 hasConceptScore W2029567090C162711632 @default.
• W2029567090 hasConceptScore W2029567090C184779094 @default.
• W2029567090 hasConceptScore W2029567090C185592680 @default.
• W2029567090 hasConceptScore W2029567090C41999313 @default.
• W2029567090 hasConceptScore W2029567090C62520636 @default.

• next