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• W2029657911 abstract "The adsorption of CO on Cu(111) has been re-investigated using Fourier transform reflection absorption infrared spectroscopy (FT-RAIRS), electron energy loss spectroscopy (EELS) and low energy electron diffraction (LEED). The combination of these techniques has revealed important new information about this system. At 95 K three adsorption stages (1 to 3) can be distinguished, leading to successive ordered overlayer structures (I to III). Stage 1 exists for coverages up to 0.33 and involves linearly bound species only. The sharpest band observed during the course of these experiments, with an intrinsic FWHM of 4.5 cm−1, is associated with a coverage of 0.33 and an ordered (√3 × √3)R30 ° structure (I). Stage 2 is associated with the coverage regime 0.33−0.44. In this stage EELS data show tilted, linear CO species are present. No bridged species exist at this point. On the basis of this, we propose a new overlayer structure (II), for θ = 0.44. Increasing the coverage gives stage 3. During this process, the high resolution FT-RAIRS spectra resolved two bands associated with linear CO species. The behaviour of these bands suggests that the final structure (III) is formed in a step-wise manner, with islands of (II) and (III) coexisting in the adlayer. Both linear and bridged species exist in stage 3. The bandshapes suggest significant inhomogeneities in the adlayer are present at the saturation coverage. Finally, the concentration of bridged species is found to be very sensitive to the adsorption temperature." @default.
• W2029657911 created "2016-06-24" @default.
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• W2029657911 date "1988-09-01" @default.
• W2029657911 modified "2023-10-18" @default.
• W2029657911 title "FT-rairs, eels and leed studies of the adsorption of carbon monoxide on Cu(111)" @default.
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• W2029657911 doi "https://doi.org/10.1016/0039-6028(88)90088-x" @default.
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