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• W2029659426 startingPage "6884" @default.
• W2029659426 abstract "The first application of the Pauson–Khand reaction (PKR) to the synthesis of azabridged bicyclic structures is described. Compounds containing azabicyclo[3.3.1]nonane and azabicyclo[3.2.1]octane rings fused to cyclopentenones were efficiently constructed via the PKR of cis-2,6-disubstituted N-acyl piperidine enyne substrates, many of which can be readily prepared from 4-methoxypyridine in a few steps. Moreover, the PKR of cis-2,6-disubstituted piperazine enynes allowed the preparation of diazabicyclo[3.3.1]nonanes fused to cyclopentenones. This new strategy for the synthesis of azabridged bicyclic frameworks was exploited as a key step in a concise, enantioselective total synthesis of the macroline alkaloid (−)-alstonerine." @default.
• W2029659426 created "2016-06-24" @default.
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• W2029659426 date "2008-07-01" @default.
• W2029659426 modified "2023-10-16" @default.
• W2029659426 title "The Pauson–Khand reaction as a new entry to the synthesis of bridged bicyclic heterocycles: application to the enantioselective total synthesis of (−)-alstonerine" @default.
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• W2029659426 doi "https://doi.org/10.1016/j.tet.2008.02.066" @default.
• W2029659426 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/2516352" @default.
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