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- W2029778924 abstract "Recent experiments show that supercooled liquids around the glass transition temperature are dynamically heterogeneous [H. Sillescu, J. Non-Cryst. Solids 243, 81 (1999)]. Such heterogeneity is expected from the random first order transition theory of the glass transition. Using a microscopic approach based on this theory, we derive a relation between the departure from Debye relaxation as characterized by the beta value of a stretched exponential response function, phi(t) = e(-(t/tau(KWW))beta), and the fragility of the liquid. The beta value is also predicted to depend on temperature and to vanish as the ideal glass transition is approached at the Kauzmann temperature." @default.
- W2029778924 created "2016-06-24" @default.
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- W2029778924 date "2001-06-11" @default.
- W2029778924 modified "2023-10-14" @default.
- W2029778924 title "Microscopic Theory of Heterogeneity and Nonexponential Relaxations in Supercooled Liquids" @default.
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- W2029778924 doi "https://doi.org/10.1103/physrevlett.86.5526" @default.
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