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- W2030051019 abstract "Optical, spin resonance, and high-field magnetoresistance studies of the organic charge-transfer salt ${(mathrm{tetrathiatetracene})}_{2}$${(mathrm{iodide})}_{3}$ [${(mathrm{TTT})}_{2}$${mathrm{I}}_{3}$] have been carried out. This material is a single-carrier system consisting of segregated linear chains of TTT cation radicals and tri-iodide ions which are incommensurate with respect to each other. The ${mathrm{I}}_{3}^{ensuremath{-}}$ chains exhibit considerable disorder perpendicular to the chain axis. ${(mathrm{TTT})}_{2}$${mathrm{I}}_{3}$ has a high room-temperature conductivity $ensuremath{sigma}(300ifmmode^circelsetextdegreefi{}mathrm{K})ensuremath{sim}1000$ ${mathrm{ensuremath{Omega}}}^{ensuremath{-}1}$${mathrm{cm}}^{ensuremath{-}1}$ along the chain axis and is metallic down to ensuremath{sim}100ifmmode^circelsetextdegreefi{}K where a possible phase transition occurs. The nature of this transition is discussed. Below 30ifmmode^circelsetextdegreefi{}K, ${(mathrm{TTT})}_{2}$${mathrm{I}}_{3}$ exhibits semiconducting properties indicating that the low-temperature ground state is nonmetallic." @default.
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- W2030051019 date "1978-04-01" @default.
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- W2030051019 title "Optical, spin-resonance, and magnetoresistance studies of(tetrathiatetracene)2(iodide)3. The nature of the ground state" @default.
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- W2030051019 doi "https://doi.org/10.1103/physrevb.17.2853" @default.
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