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- W2030144061 abstract "The oxidation of 7,9-dimethyluric acid by H2O2; catalyzed by type VIII peroxidase (from horseradish peroxidase) has been studied and the results obtained compared to previous studies on the electrochemical oxidation mechanism. At the pH values studied (3–5 and 7–9) the enzymatic oxidation generates intermediate species which are identical to those formed in the peak Ia electrochemical oxidation reaction. At high pH (7–9), where 7,9-dimethyluric acid is a monoanion, the products formed in the peroxidase-catalyzed reaction are 1,3-dimethylallantoin, and 1-hydroxy-2,4-dimethyl-2,4,6,8-tetraaza-3,7-dioxo-5-ene-bicyclo-(3.3.0)-octane. These are the products formed as a result of the peak Ia plus peak IIa electrooxidation reactions. At lower pH (3–5) the products formed in the peroxidase-catalyzed reaction are 1,3-dimethylallantoin and 1,3-dimethyl-5-hydroxyhydantoin-5-carboxamide. The intermediates and products formed in the enzymatic reaction are exactly the same as are observed in the peak Ia electrochemical oxidation. Accordingly, it has been concluded that the enzymatic and electrochemical processes proceed by very similar, if not identical, chemical reaction pathways." @default.
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- W2030144061 date "1983-10-01" @default.
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- W2030144061 title "Peroxidase-catalyzed oxidation of 7,9-dimethyluric acid" @default.
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- W2030144061 doi "https://doi.org/10.1016/0302-4598(83)85102-2" @default.
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