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- W2030228061 abstract "Conventional high-yielding reactions (such as etherification, condensation reactions) and palladium-catalysed aminocarbonylation served as highly efficient synthetic tools for the synthesis of novel cavitands bearing Schiff-base and carboxamide/2-ketocarboxamide functionalities, respectively. In this way, two families of deepened cavitands with related structures possessing 2-, 3- and 4-picolylamine moieties on the upper rim have been synthesised. Unexpectedly high chemoselectivities towards tetracarboxamides and tetrakis(2-ketocarboxamides) have been observed. The aminocarbonylation of tetraiodocavitand as an iodoaromatic substrate proved to be highly selective in two aspects: (i) no substantial formation of either the mono-, di- or trifunctionalized products was observed and (ii) no ‘mixed’ products possessing both carboxamide and 2-ketocarboxamide fragments, due to selective simple and double carbon monoxide insertion, were detected." @default.
- W2030228061 created "2016-06-24" @default.
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- W2030228061 date "2015-04-01" @default.
- W2030228061 modified "2023-10-03" @default.
- W2030228061 title "High-yielding synthesis of deepened cavitands bearing picolyl moieties on the upper rim" @default.
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- W2030228061 doi "https://doi.org/10.1016/j.tet.2015.03.009" @default.
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