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- W2030541755 abstract "The distribution details of strongly-localized fields in metal nanostructures are important for strong interaction with the locally-varying non-linearity. Using gold nanodimers with nanogaps, we demonstrate that field localization alone is insufficient to drive a strong second-order response. Instead, polarization conversion of the local fundamental field combines with its asymmetric distribution along the dimer perimeter to yield strong responses. Strongly-localized fields may also favor higher-multipole (magnetic-dipole and electric-quadrupole) contributions to their nonlinear response. We show that the polarization-dependent interference of multipole sources in second-harmonic generation from gold nanoparticles allows the separation of their relative contributions." @default.
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- W2030541755 date "2007-09-01" @default.
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- W2030541755 title "LOCAL-FIELD AND MULTIPOLAR EFFECTS IN THE SECOND-HARMONIC RESPONSE OF ARRAYS OF METAL NANOPARTICLES" @default.
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- W2030541755 doi "https://doi.org/10.1142/s0218863507003809" @default.
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