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• W2030580274 abstract "Temperature-dependent rf-ion trap mass spectrometry and first-principles simulations reveal the detailed reaction mechanism of the catalytic gas-phase oxidation of CO by free Au(2)(-) ions in the presence of O(2). A metastable intermediate with a mass of Au(2)CO(3)(-) was observed at low temperatures. Two alternative structures corresponding to digold carbonate or peroxyformate are predicted for this intermediate. Both structures are characterized by low activation barriers for the formation of CO(2). These combined experimental and theoretical investigations provide a comprehensive understanding of the kinetics, energetics, and atomic arrangements along the reaction path, thus allowing a formulation of the catalytic cycle for the oxidation reaction." @default.
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• W2030580274 date "2003-08-01" @default.
• W2030580274 modified "2023-10-14" @default.
• W2030580274 title "Catalytic CO Oxidation by Free Au₂^-: Experiment and Theory" @default.
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• W2030580274 doi "https://doi.org/10.1021/ja027926m" @default.
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