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- W2030773368 abstract "The quantum‐mechanical theory of vibronic dephasing presented in the first paper of this series is applied to the case of a diatomic impurity dissolved in a solid rare‐gas host. An explicit expression for the pure dephasing rate T2′−1 is derived in terms of microscopic properties of the impurity and host, and the effects of variations in the parameters characterizing these properties are investigated. The expression for T2′−1 is applied specifically to the system Cl2/Ar in order to relate the results to those of previous classical‐trajectory calculations and of experimental measurements. The significance of anharmonicity in the intramolecular potential curve (of the impurity) is demonstrated." @default.
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- W2030773368 date "1979-01-01" @default.
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- W2030773368 title "Vibronic dephasing of anharmonic molecules. II. Impurity molecules isolated in low-temperature matrices" @default.
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- W2030773368 doi "https://doi.org/10.1063/1.438718" @default.
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