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- W2030903543 abstract "A hierarchical meso/macroporous zeolite-supported Co catalyst (Co/ASB) was designed and employed for the direct synthesis of isoparaffins. The hierarchical porous zeolite (ASB) was developed by a steam-assisted crystallization method using alumina-modified meso/macroporous silica as the precursor. Structural characterization indicated that the as-synthesized ASB exhibited nanosized β-zeolite crystallites and a hierarchical meso/macroporous structure. The activity of the Co/ASB catalyst was much higher than that of conventional Co catalysts supported on SiO2 (Co/SiO2) and H-β-zeolite (Co/B). A high isoparaffins selectivity of 30.5 % was obtained from Co/ASB because of the hydrocracking/isomerization of long-chain hydrocarbons at the strong acidic sites of the β-zeolite. Furthermore, as a result of the fast diffusion of syngas in the unique hierarchical pores, the methane selectivity of Co/ASB was lower than that of Co/B." @default.
- W2030903543 created "2016-06-24" @default.
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- W2030903543 date "2015-01-30" @default.
- W2030903543 modified "2023-09-27" @default.
- W2030903543 title "Design of a Hierarchical Meso/Macroporous Zeolite-Supported Cobalt Catalyst for the Enhanced Direct Synthesis of Isoparaffins from Syngas" @default.
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- W2030903543 doi "https://doi.org/10.1002/cctc.201402929" @default.
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