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- W2031004957 abstract "Liquid cell electron microscopy enables direct in situ imaging of processes in liquids and objects suspended in liquids with nanoscale resolution. However, the irradiating electrons affect the chemistry of the suspending medium, typically an aqueous solution, producing molecular and radical products such as hydrogen, oxygen, and hydrated (solvated) electrons. These may impact the imaged structures and phenomena. A good understanding of the interactions between the electrons and the irradiated medium is necessary to correctly interpret experiments, minimize artifacts, and take advantage of the irradiation. We predict the composition of water subjected to electron irradiation in the electron microscope. We reinterpret available experimental data, such as beam-induced variations in pH and colloid aggregation, in light of our predictions and show new observations of crystallization and etching as functions of dose rate, resolving conflicting reports in the scientific literature. We make our computer code avai..." @default.
- W2031004957 created "2016-06-24" @default.
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- W2031004957 date "2014-09-11" @default.
- W2031004957 modified "2023-10-17" @default.
- W2031004957 title "Electron–Water Interactions and Implications for Liquid Cell Electron Microscopy" @default.
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- W2031004957 doi "https://doi.org/10.1021/jp507400n" @default.
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