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• W2031065024 abstract "It is shown how the effects of molecular reorientation may be incorporated in a fully quantized quantum-electrodynamical treatment of a high-order nonlinear optical effect. Specifically, a general temporal theory is developed to account for the second-harmonic intensity produced through phase-conjugate six-wave mixing. The theory permits elucidation of the intensity of the second-harmonic radiation for arbitrary arrangements of the generating laser beams and molecular geometry. Several models are considered: a one-dimensional model, linear geometry, and a planar geometry. A comparison is made between the results associated with these models and with those obtained from ultrafast experiments on dilute solutions of substituted stilbenes. We find that the off-axial components of the molecular polarizabilities are necessary to properly describe the orientational dynamics of such molecules." @default.
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• W2031065024 date "2000-07-18" @default.
• W2031065024 modified "2023-09-27" @default.
• W2031065024 title "Quantum-electrodynamical treatment of second-harmonic generation through phase-conjugate six-wave mixing: Temporal analysis" @default.
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• W2031065024 doi "https://doi.org/10.1103/physreva.62.023807" @default.
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