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- W2031077179 abstract "The melting-point depression of a random copolymer with comonomer exclusion from the crystalline phase is investigated. The analysis is based on simulation results obtained with an extended Sadler-Gilmer crystallization model. Apparent copolymer melting points Tcopm(l) of lamellae of finite thickness l are observed. Further thickening is entropically suppressed. It is shown that the average lamellar thickness and the minimum thermodynamically stable thickness converge at Tcopm. The fine-grained nature of the model reveals an entropic contribution to the melting-point depression, which is due to the so-called blind attachment of chain segments to the growth face. Our new ‘kinetic’ melting-point equation is compared with the ‘equilibrium’ result by Flory and shows a considerably stronger melting-point depression." @default.
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- W2031077179 date "1992-01-01" @default.
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- W2031077179 title "On the melting-point depression of copolymer crystals" @default.
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- W2031077179 doi "https://doi.org/10.1016/0032-3861(92)90336-u" @default.
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