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- W2031141245 abstract "The kinetics of the sequestration of iron(III) from the polynuclear iron(III) complex, [Fe11O6(OH)6(O2CPh)15]· H2O·2MeCN, a possible biomimetic model of ferritin, with a series of 11 primary and secondary hydroxamic acids in dry acetonitrile/dichloromethane solvent mixtures indicates an associative interchange (Ia) mechanism in accordance with the wide variation of ΔH⧧ and ΔS⧧ within the series. Comparison of the kinetics of this hydroxamic acid series with the simple binuclear iron complex (NEt4)2[Fe2OC16] shows that steric effects are considerably more important for the Fe11 complex than for the Fe2 complex. These conclusions, based on kinetics studies, are relevant to the design of chelators for sequestration of iron from ferritin." @default.
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- W2031141245 date "1999-10-29" @default.
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- W2031141245 title "Kinetics of Iron(III) Chelation from Polynuclear Oxo-Hydroxy Aggregates by Hydroxamic Acids: Understanding Ferritin Iron(III) Sequestration" @default.
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- W2031141245 doi "https://doi.org/10.1021/ic990158o" @default.
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