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- W2031413197 abstract "We argue that a transient size calibration of self-assembled nanoparticles during strained epitaxy can be caused by forces interior to the growing islands without substrate-propagated interparticle interactions or intermixing with the substrate. The role of substrate in our mechanism is only to provide the intraparticle elastic strain. Our arguments are based on kinetic Monte Carlo simulations of the $(1+1)$-dimensional model of strained epitaxy of Ratsch and Zangwill (RZ) [Surf. Sci. 293, 123 (1993)]. It has been found that while the energetics of the RZ model predicts indefinite ripening of the islands, in the simulations their linear dimensions saturated at intermediate times near some finite coverage-dependent values. Simultaneously statistical distributions of their widths and heights narrowed, thus providing improved size calibration. The size distributions obtained are qualitatively similar to those observed experimentally in the growth of ultrasmall supported metallic clusters. The applicability of the model to such systems is briefly discussed." @default.
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- W2031413197 date "2005-07-14" @default.
- W2031413197 modified "2023-09-26" @default.
- W2031413197 title "Size calibration of self-assembled nanoparticles in a model of strained epitaxy with passive substrate" @default.
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- W2031413197 doi "https://doi.org/10.1103/physrevb.72.035438" @default.
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