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- W2031566978 abstract "Relations between the structure and low-frequency excitations (LFEs) which dominate the dynamics at low temperatures were investigated in lithiumsilicophosphate glasses by means of nuclear magnetic resonance (NMR), electrical conductivity and X-ray photoelectron spectroscopy (XPS). By varying the glass composition we observed three different kinds of LFEs which could be analyzed consistently by an asymmetric double well potential (ADWP) approach. We were able to link the different LFEs with structural units of the glasses detected by magic angle spinning NMR and XPS. In particular, [SiO6]2− units are shown to be connected to LFEs caused by charge fluctuations of Li+ ions, whereas fluctuations of neutral [PO4]0 units are found to be the source of the two other LFEs." @default.
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- W2031566978 date "1997-12-01" @default.
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- W2031566978 title "Structural basis of low-frequency excitations in silicophosphate glasses" @default.
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- W2031566978 doi "https://doi.org/10.1016/s0022-3093(97)90131-9" @default.
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