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• W2031696860 abstract "Abstract Dense BaCo 0.7 Fe 0.2 Ta 0.1 O 3−δ (BCFT) perovskite membranes were successfully synthesized by a simple solid state reaction. In situ high‐temperature X‐ray diffraction indicated the good structure stability and phase reversibility of BCFT at high temperatures. The thermal expansion coefficient (TEC) of BCFT was determined to amount 1.02 × 10 −5 K −1 , which is smaller than those of Ba 0.5 Sr 0.5 Co 0.8 Fe 0.2 O 3−δ (BSCF) (1.15 × 10 −5 K −1 ), SrCo 0.8 Fe 0.2 O 3−δ (SCF) (1.79 × 10 −5 K −1 ), and BaCo 0.4 Fe 0.4 Zr 0.2 O 3−δ (BCFZ) (1.03 × 10 −5 K −1 ). It can be seen that the introduction of Ta ions into the perovskite framework could effectively lower the TEC. Thickness dependence studies of oxygen permeation through the BCFT membrane indicated that the oxygen permeation process was controlled by bulk diffusion. A membrane reactor made from BCFT was successfully operated for the partial oxidation of methane to syngas at 900°C for 400 h without failure and with the relatively high, stable oxygen permeation flux of about 16.8 ml/min cm 2 . © 2009 American Institute of Chemical Engineers AIChE J, 2010" @default.
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• W2031696860 date "2009-08-24" @default.
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• W2031696860 title "Oxygen permeability and structural stability of a novel tantalum-doped perovskite BaCo_0.7Fe_0.2Ta_0.1O3−<i>δ</i>" @default.
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• W2031696860 doi "https://doi.org/10.1002/aic.12044" @default.
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