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- W2031738196 abstract "Abstract On the basis of one-electron Hartree-Fock approximation, the extended-ion method has been used to investigate desorption induced by the formation and trapping of two types of excitons on and near the three different faces ((100), (110), (111)) for solid Ne and Kr. Excited Ne atom, Ne excimer and Kr excimer can be ejected upon self-trapping of excitons on and near the surface, while excited Kr atom cannot. After desorption, the excited atom and excimer will decay radiatively, the luminescence energies are in fair agreement with the experiment. For the excimer, the radiative decay terminates at the strongly repulsive ground state, this repulsive energy is converted into kinetic energy of two atoms constituting the excimer, resulting in the desorption of ground state atom. It is also observed that a localized hole on the surface and below is efficiently converted into a molecule-ion R2+ without leading to any desorption, showing that exciton-lattice interaction plays a key role in the process of desorption. The ejected direction is basically along the normal to the surface for the excited particle, but for the ground state atom, it does not show a preferential direction of desorption." @default.
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- W2031738196 date "1996-08-01" @default.
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- W2031738196 title "Desorption of atoms and excimers upon self-trapping of excitons in rare gas solids" @default.
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- W2031738196 doi "https://doi.org/10.1016/0168-583x(96)00120-6" @default.
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