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- W2031896178 abstract "Product analyses and nanosecond time-resolved spectroscopy on laser flash photolysis were studied for the photoinduced electron-transfer reaction of 3,4-di(alpha-styryl)furan (6a). A combination of these results, kinetic, density functional theoretical (DFT), and time-dependent DFT analyses enabled assignment of the absorption to the tetramethyleneethane (TME)-type radical cation (7a*+, lambda(max) = 392 nm) and the corresponding singlet biradical ((1)7a**, lambda(max) = 661 nm). These two intermediates were mechanistically linked to each other with a facile back electron-transfer reaction. The present studies provide a new method for the generation of aryl-substituted TME-type intermediates." @default.
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- W2031896178 date "2008-02-01" @default.
- W2031896178 modified "2023-10-18" @default.
- W2031896178 title "The Facile Generation of a Tetramethyleneethane Type Radical Cation and Biradical Utilizing a 3,4-Di(α-styryl)furan and a Photoinduced ET and Back ET Sequence" @default.
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- W2031896178 doi "https://doi.org/10.1021/ja074000b" @default.
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