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- W2032010410 abstract "Correlation enhancement of electrons in Ni nano-clusters due to confinement in reduced dimensions has been observed. Both the size and shape of the nano-clusters have a strong influence on the Ni 2p satellite structures. For small Ni clusters, apart from the 6 eV satellite, a 3 eV satellite structure emerges in Ni 2p3/2 photoemission spectra due to the existence of the 3F atomic state. However, the intensity of the 3 eV satellite decreases with increasing cluster size because the Ni 3d level becomes increasingly occupied in large clusters. The increased electron population in the 3d level is achieved through electron transfer from the free-electron-like 4sp states to the unhybridized pure 3d spin down states; the latter is lower in energy than the 3d–4sp hybridized states. The correlation-induced 6 eV satellite energy is enhanced by Ar+ bombardment. These observations make it feasible to gauge the Ni 3d electron population by probing the 2p photoemission spectra and to modify the supported Ni nano-clusters through thermal treatment and/or ion bombardment." @default.
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- W2032010410 date "2008-10-17" @default.
- W2032010410 modified "2023-10-18" @default.
- W2032010410 title "Evolution of the 2p satellite of Ni nano-clusters on TiO2(001) surfaces" @default.
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