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- W2032019297 abstract "Recently, we proposed a new four-parametric MGAB equation (modified Guggenheim–Anderson–De Boer equation, GAB) for fitting of experimental isotherms of vapor-phase sorption on geosorbents. In the present study, the theoretical meaning of MGAB equation was elucidated. For this purpose, the properties of the equation of multilayer adsorption on a heterogeneous surface with local characteristics described by GAB model and Zeldovitsh–Roginskiy energy distribution function ρ ( ɛ ) were derived and the satisfaction of MGAB equation with these properties was shown. MGAB model has two parameters connected with GAB model: v m is the monolayer sorption capacity and k is the constant of the multilayer sorption, as well as two parameters of sorption energy distribution function ρ ( ɛ ): α , characterizing heterogeneity of ρ ( ɛ ) and C 0 , reflecting energy baseline. The influence of parameters α and C 0 on the shape of both ρ ( ɛ ) and model sorption isotherm was established. The applicability of MGAB model for the description of surface heterogeneity of a natural sorbent by example of 13 different sorbate–sorbent systems dried and moistened has been discussed. For these systems equilibrium sorption isotherms were measured, corresponding energy distribution functions ρ ( ɛ ) were calculated, and obtained α values were compared. On the whole, the differences in α values responded to the real tendencies of heterogeneity changes in these systems." @default.
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- W2032019297 date "2007-03-01" @default.
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- W2032019297 title "The equation of vapor-phase sorption on heterogeneous surfaces with local Guggenheim–Anderson–De Boer model" @default.
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- W2032019297 doi "https://doi.org/10.1016/j.colsurfa.2006.09.043" @default.
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